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Open Quantum Systems Decoherence Quantum Chemistry

Theory of vibronic assistance in the nonequilibrium condensation of exciton polaritons in optically--pumped organic single crystal microcavities

arXiv

Authors: Eric R. Bittner, Svitlana Zaster, Carlos Silva

Year

2012

Paper ID

8620

Status

Preprint

Abstract Read

~2 min

Abstract Words

105

Citations

N/A

Abstract

We present a reaction/diffusion model for the formation of a lower polariton condensate in a micro cavity containing an organic semiconducting molecular crystalline film. Our model--based upon an anthracene film sandwiched between two reflecting dielectric mirrors--consists of three coupled fields corresponding to a gas of excitons created by an external driving pulse, a reservoir of vibron states formed by the coupling between a ground-state vibrational model and a cavity photon, and a lower polariton condensate. We show that at finite temperature, the presence of the vibron reservoir can augment the exciton population such that a lower critical pumping threshold is required to achieve condensation.

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We present a reaction/diffusion model for the formation of a lower polariton condensate in a micro cavity containing an organic semiconducting molecular crystalline film.

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References & Citation Signals

[1] DOI https://doi.org/arXiv:1206.2906 [2] arXiv https://arxiv.org/abs/1206.2906 [3] Publisher https://arxiv.org/abs/1206.2906

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