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Quantum Chemistry
Laser-induced bound-state phases in high-order harmonic generation
arXiv
Authors: Adam Etches, Mette B. Gaarde, Lars Bojer Madsen
Year
2012
Paper ID
8678
Status
Preprint
Abstract Read
~2 min
Abstract Words
60
Citations
N/A
Abstract
We present single-molecule and macroscopic calculations showing that laser-induced Stark shifts contribute significantly to the phase of high-order harmonics from polar molecules. This is important for orbital tomography, where phases of field-free dipole matrix elements are needed in order to reconstruct molecular orbitals. We derive an analytical expression that allows the first-order Stark phase to be subtracted from experimental measurements.
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- This paper contributes to the Quantum Chemistry research area in the Quantum Articles archive.
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- We present single-molecule and macroscopic calculations showing that laser-induced Stark shifts contribute significantly to the phase of high-order harmonics from polar molecules.
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