Analog quantum simulation of Shastry-Sutherland Ising materials

Frustrated magnets host rich emergent behavior because competing interactions generate dense manifolds of low-energy states. The Ising Shastry-Sutherland model is a paradigmatic setting, motivated experimentally by Ising-like rare-earth tetraborides such as TmB₄ and ErB₄, whose field-induced magnetization plateaus have motivated extensive microscopic modeling. Yet how tunable quantum fluctuations reorganize this material-motivated phase diagram remains largely unexplored. Here, we realize a transverse- and longitudinal-field Ising model on the Shastry-Sutherland lattice using a programmable Rydberg-atom array. We map its quantum phase diagram using density matrix renormalization group calculations and probe corresponding signatures experimentally in arrays containing more than 110 atoms. Beyond the established classical phases, the calculations identify two regimes absent in the classical limit and stabilized at finite transverse field: a 2/5 filling plateau whose finite stability region emerges from a classically degenerate phase boundary and a symmetry-preserving quantum-dimer regime replacing classically selected collinear order. Experiments on finite open arrays reveal signatures consistent with these regimes across three boundary-pinning conditions, with the resulting response maps agreeing qualitatively with the calculated phase diagram. Our results establish programmable Rydberg-atom arrays as tools for exploring frustrated, material-motivated Hamiltonians and motivate searches for new, quantum-driven magnetization plateaus and quantum-dimer behavior in ErB₄ under a transverse field or in strain-tuned TmB₄.