Optimized Tensor-Network Renormalization for Quantum Dynamics: Resolving the Spectral Function of K_2Co\(SeO₃\)₂

Tensor-network methods have opened a powerful route for the study of dynamical spectral functions in two-dimensional quantum systems. However, existing approaches within the framework of infinite projected entangled-pair states construct the required renormalization tensors solely from the ground-state environment and can suffer from severe numerical instability. We identify the origin of this instability and introduce an excitation-tailored corner-transfer-matrix renormalization-group (ET-CTMRG) method to resolve it. By incorporating excitation tensors into the renormalization procedure, the method constructs a substantially more accurate effective Hamiltonian matrix and thereby yields reliable and well-converged excitation spectra. For Heisenberg antiferromagnets, it reduces truncation errors by orders of magnitude and for the particularly complex case of the supersolid phase in the triangular-lattice XXZ magnet K_2Co\(SeO₃\)₂, it achieves excellent quantitative agreement with inelastic neutron-scattering measurements. ET-CTMRG therefore provides a robust framework for investigating the dynamical properties of strongly correlated quantum systems.