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Photoelectron spectroscopy with a resonant dichromatic field: Role of geometric phase
arXiv
Authors: Evan Munaro-Langloÿs, Axel Stenquist, Jan Marcus Dahlström
Year
2026
Paper ID
67861
Status
Preprint
Abstract Read
~2 min
Abstract Words
195
Citations
N/A
Abstract
We investigate geometric-phase control in resonantly driven two-level atoms exposed to near-degenerate dichromatic laser pulses. In contrast to conventional two-color schemes based on widely separated frequencies, the closely spaced frequency components generate a slowly varying beating envelope that repeatedly reverses the pseudo-spin rotation on the Bloch sphere. This enables coherent control of the geometric phase accumulated during Rabi dynamics and strongly modifies the resulting photoelectron spectra. Using an exactly solvable model for flat-top pulse envelopes, we derive the essential-state dynamics analytically and analyze photoionization induced both by an auxiliary field and by the dichromatic driving field itself. We show that the formation of Autler--Townes doublets can be interpreted in terms of destructive interference associated with geometric phases acquired during completed pseudo-spin rotations. Beyond the canonical Autler--Townes regime, beat-induced reversal dynamics lead to qualitatively different spectral structures, including re-emergent central peaks and higher-order sidebands. These effects originate from the nonuniform temporal evolution induced by the beating envelope, which modifies the balance between positive and negative excitation amplitudes. Our results establish beating-field control as a route toward engineering geometric-phase interference in ultrafast light--matter interactions and suggest broader applications in coherent control of atoms, molecules, and x-ray-driven systems.
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- This paper contributes to the Quantum Chemistry research area in the Quantum Articles archive.
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- We investigate geometric-phase control in resonantly driven two-level atoms exposed to near-degenerate dichromatic laser pulses.
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