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Open Quantum Systems Decoherence

The connection between time-local and time-nonlocal perturbation expansions

arXiv
Authors: K. Nestmann, M. R. Wegewijs

Year

2021

Paper ID

63098

Status

Preprint

Abstract Read

~2 min

Abstract Words

203

Citations

N/A

Abstract

There exist two canonical approaches to describe open quantum systems by a time-evolution equation: the Nakajima-Zwanzig quantum master equation, featuring a time-nonlocal memory kernel mathcal{K}, and the time-convolutionless equation with a time-local generator mathcal{G}. These key quantities have recently been shown to be connected by an exact fixed-point relation [Phys. Rev. X 11, 021041 (2021)]. Here we show that this implies a recursive relation between their perturbative expansions, allowing a series for the kernel mathcal{K} to be translated directly into a corresponding series for the more complicated generator mathcal{G}. This leads to an elegant way of computing the generator using well-developed, standard memory-kernel techniques for strongly interacting open systems. Moreover, it allows for an unbiased comparison of time-local and time-nonlocal approaches independent of the particular technique chosen to calculate expansions of mathcal{K} and mathcal{G} (Nakajima-Zwanzig projections, real-time diagrams, etc.). We illustrate this for leading and next-to-leading order calculations of mathcal{K} and mathcal{G} for the single impurity Anderson model using both the bare expansion in the system-environment coupling and a more advanced renormalized series. We compare the different expansions obtained, quantify the legitimacy of the generated dynamics (complete positivity) and benchmark with the exact result in the non-interacting limit.

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  • There exist two canonical approaches to describe open quantum systems by a time-evolution equation: the Nakajima-Zwanzig quantum master equation, featuring a time-nonlocal...

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