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Hyperfine spectroscopy of optical-cycling transitions in singly ionized thulium

arXiv
Authors: Patrick Müller, Andrei Tretiakov, Amanda Younes, Nicole Halawani, Paul Hamilton, Wesley C. Campbell

Year

2025

Paper ID

6035

Status

Preprint

Abstract Read

~2 min

Abstract Words

107

Citations

N/A

Abstract

We present a spectroscopic investigation of 169Tm^+ that provides two key foundations for its use as a platform for advanced quantum applications. First, we establish the complete spectroscopic road map for optical cycling (including laser cooling) by performing high-resolution spectroscopy on 169Tm^+ ions in an ion trap. We characterize the primary 313 nm and complementary 448/453 nm cycling transitions, identify the essential near-infrared repumping frequencies, and determine the magnetic-dipole hyperfine A constants for all relevant levels. Second, we report detailed characterization of a metastable state as a candidate for hosting a robust qubit, performing lifetime measurements and Zeeman-resolved microwave hyperfine spectroscopy with kHz precision.

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  • We present a spectroscopic investigation of ^169Tm^+ that provides two key foundations for its use as a platform for advanced quantum applications.

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