Coherent control of a nuclear spin via interactions with a rare-earth ion in the solid-state

Individually addressed Er³⁺ ions in solid-state hosts are promising resources for quantum repeaters, because of their direct emission in the telecom band and compatibility with silicon photonic devices. While the Er³⁺ electron spin provides a spin-photon interface, ancilla nuclear spins could enable multi-qubit registers with longer storage times. In this work, we demonstrate coherent coupling between the electron spin of a single Er³⁺ ion and a single I=1/2 nuclear spin in the solid-state host crystal, which is a fortuitously located proton $¹$H. We control the nuclear spin using dynamical decoupling sequences applied to the electron spin, implementing one- and two-qubit gate operations. Crucially, the nuclear spin coherence time exceeds the electron coherence time by several orders of magnitude, because of its smaller magnetic moment. These results provide a path towards combining long-lived nuclear spin quantum registers with telecom-wavelength emitters for long-distance quantum repeaters.