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Trapped Ion Quantum Computing
Quantum Chemistry
Energy-scaling of the product state distribution for three-body recombination of ultracold atoms
arXiv
Authors: Shinsuke Haze, José P. D'Incao, Dominik Dorer, Jinglun Li, Markus Deiß, Eberhard Tiemann, Paul S. Julienne, Johannes Hecker Denschlag
Year
2022
Paper ID
57591
Status
Preprint
Abstract Read
~2 min
Abstract Words
191
Citations
N/A
Abstract
Three-body recombination is a chemical reaction where the collision of three atoms leads to the formation of a diatomic molecule. In the ultracold regime it is expected that the production rate of a molecule generally decreases with its binding energy Eb, however, its precise dependence and the physics governing it have been left unclear so far. Here, we present a comprehensive experimental and theoretical study of the energy dependency for three-body recombination of ultracold Rb. For this, we determine production rates for molecules in a state-to-state resolved manner, with the binding energies Eb ranging from 0.02 to 77 GHztimes h. We find that the formation rate approximately scales as Eb-α, where α is in the vicinity of 1. The formation rate typically varies only within a factor of two for different rotational angular momenta of the molecular product, apart from a possible centrifugal barrier suppression for low binding energies. In addition to numerical three-body calculations we present a perturbative model which reveals the physical origin of the energy scaling of the formation rate. Furthermore, we show that the scaling law potentially holds universally for a broad range of interaction potentials.
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- This paper contributes to the Quantum Chemistry research area in the Quantum Articles archive.
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- Three-body recombination is a chemical reaction where the collision of three atoms leads to the formation of a diatomic molecule.
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