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Open Quantum Systems Decoherence Quantum Chemistry

Optical Regulation of Chiral-Induced Spin Selectivity

arXiv

Authors: Wei Liu, Jingqi Chen, Wenjie Dou

Year

2023

Paper ID

53747

Status

Preprint

Abstract Read

~2 min

Abstract Words

103

Citations

N/A

Abstract

We present a non-perturbative theory that describes how light regulates chiral-induced spin selectivity (CISS) from the perspective of strong light-matter interactions. The research results indicate that 1) light can have opposite effects on the CISS, 2) the difference in CISS is caused by the steady states of nuclei coupled to spin electrons and 3) this steady state differences are caused by the different light-induced Lorentz forces felt by spin-up and spin-down electrons. The fundamental reason for these results is the impact of light on spin-orbital coupling (SOC), which is a complex process. This theoretical framework is verified by the calculations of Floquet SOC non-adiabatic nuclear dynamics.

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We present a non-perturbative theory that describes how light regulates chiral-induced spin selectivity (CISS) from the perspective of strong light-matter interactions.

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References & Citation Signals

[1] DOI https://doi.org/arXiv:2310.10929 [2] arXiv https://arxiv.org/abs/2310.10929 [3] Publisher https://arxiv.org/abs/2310.10929

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