Quantum Fisher Information as a Thermal and Dynamical Probe in Frustrated Magnets: Insights from Quantum Spin Ice

Quantum Fisher information (QFI) is a novel measure of multipartite quantum entanglement that can be measured in inelastic neutron scattering experiments on quantum magnets. In this work, we demonstrate that the QFI can be used to understand the thermal and dynamical properties of quantum magnets by focusing on the pyrochlore lattice model of quantum spin ice (QSI), a three-dimensional quantum spin liquid that hosts fractionalized quasiparticles and emergent photons. We use the newly developed multi-directed loop update quantum Monte Carlo (QMC) algorithm and exact diagonalization (ED) to compute the QFI, which is further utilized to calibrate the gauge mean-field theory results. We show that the temperature and momentum dependence of the QFI can reveal characteristic energy scales of distinct phases and phase transitions in the global phase diagram. In particular, the QFI can clearly distinguish the ferromagnetic ordered phase, the thermal critical region above it, as well as two distinct QSI phases, namely zero-flux and π-flux QSI. Moreover, the QFI shows two crossover temperature scales, one from the trivial paramagnet to the classical spin ice regime and a lower temperature crossover to QSI. We discuss our results, especially for the π-flux QSI, in light of the ongoing experimental efforts on Cerium-based pyrochlore systems. Our results demonstrate that the QFI not only detects entanglement properties but can also be viewed as a sensitive thermal and dynamical probe in the investigation of quantum magnets.