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Open Quantum Systems Decoherence Quantum Simulation Quantum Chemistry

Lowest-order relativistic corrections to the fundamental limits of nonlinear-optical coefficients

arXiv
Authors: Nathan J. Dawson

Year

2014

Paper ID

47969

Status

Preprint

Abstract Read

~2 min

Abstract Words

79

Citations

N/A

Abstract

The effects of small relativistic corrections to the off-resonant polarizability, hyperpolarizability, and second hyperpolarizability are investigated. Corrections to linear and nonlinear optical coefficients are demonstrated in the three-level ansatz, which includes corrections to the Kuzyk limits when scaled to semi-relativistic energies. It is also shown that the maximum value of the hyperpolarizability is more sensitive than the maximum polarizability or second hyperpolarizability to lowest-order relativistic corrections. These corrections illustrate how the intrinsic nonlinear-optical response is affected at semi-relativistic energies.

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  • The effects of small relativistic corrections to the off-resonant polarizability, hyperpolarizability, and second hyperpolarizability are investigated.

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References & Citation Signals

[1] DOI https://doi.org/arXiv:1408.4843 [2] arXiv https://arxiv.org/abs/1408.4843 [3] Publisher https://arxiv.org/abs/1408.4843

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