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Quantum Simulation Entanglement Theory Quantum Correlations Open Quantum Systems Decoherence

Atomic correlation energies and the generalized gradient approximation

arXiv
Authors: Kieron Burke, Antonio Cancio, Tim Gould, Stefano Pittalis

Year

2014

Paper ID

47483

Status

Preprint

Abstract Read

~2 min

Abstract Words

76

Citations

N/A

Abstract

Careful extrapolation of atomic correlation energies suggests that Ec tends to -AZlog{Z} + BZ as Z tends to infinity, where Z is the atomic number, A is known, and B is about 38 milliHartrees. The coefficients roughly agree with those of the high-density limit of the real-space construction of the generalized gradient approximation. An asymptotic coefficient, missed by previous derivations, is included in a revised approximation. The exchange is also corrected, reducing atomic errors considerably.

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  • Careful extrapolation of atomic correlation energies suggests that Ec tends to -AZlogZ + BZ as Z tends to infinity, where Z is the atomic number, A is known, and B is about 38...

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