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Quantum Chemistry
Laser-Induced Electron Diffraction: Inversion of Photoelectron Spectra for Molecular Orbital Imaging
arXiv
Authors: R. Puthumpally-Joseph, J. Viau-Trudel, M. Peters, T. T. Nguyen-Dang, O. Atabek, E. Charron
Year
2016
Paper ID
42739
Status
Preprint
Abstract Read
~2 min
Abstract Words
84
Citations
N/A
Abstract
In this paper, we discuss the possibility of imaging molecular orbitals from photoelectron spectra obtained via Laser Induced Electron Diffraction (LIED) in linear molecules. This is an extension of our work published recently in Physical Review A 94, 023421 (2016) to the case of the HOMO-1 orbital of the carbon dioxide molecule. We show that such an imaging technique has the potential to image molecular orbitals at different internuclear distances in a sub-femtosecond time scale and with a resolution of a fraction of an Angström.
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- This paper contributes to the Quantum Chemistry research area in the Quantum Articles archive.
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- In this paper, we discuss the possibility of imaging molecular orbitals from photoelectron spectra obtained via Laser Induced Electron Diffraction (LIED) in linear molecules.
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