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Quantum Chemistry Open Quantum Systems Decoherence

A new channel for excitonic transport in the FMO complex

arXiv
Authors: Daniel López Díaz, Gabriel Gil, Augusto González

Year

2021

Paper ID

40439

Status

Preprint

Abstract Read

~2 min

Abstract Words

82

Citations

N/A

Abstract

We expose a new excitation transport channel in FMO, consisting of the 7 intramonomeric pigments and their 2nd nearest intermonomeric counterpart. Such a channel outcompetes the standard alternative, where intramonomeric pigments partner with their closest intermonomeric pigment. The efficient performance of the new channel lies at the interplay between incoherent energy transfer and the capacity of quantum coherence to build optimal acceptor levels. Finally, the differential fitness and peculiarity of the new over the alternative channel highlights its possible role within natural selection.

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  • We expose a new excitation transport channel in FMO, consisting of the 7 intramonomeric pigments and their 2nd nearest intermonomeric counterpart.

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