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Open Quantum Systems Decoherence
Quantum Chemistry
Emergence of Molecular Chirality by Vibrational Raman Scattering
arXiv
Authors: Farhad Taher Ghahramani, Afshin Shafiee
Year
2013
Paper ID
31889
Status
Preprint
Abstract Read
~2 min
Abstract Words
74
Citations
N/A
Abstract
In this study, we apply the monitoring master equation describing decoherence of internal states to an optically active molecule prepared in a coherent superposition of nondegenerate internal states interacting with thermal photons at low temperatures. We use vibrational Raman scattering theory up to the first chiral-sensitive contribution, i.e., the mixed electric-magnetic interaction, to obtain scattering amplitudes in terms of molecular polarizability tensors. The resulting density matrix is used to obtain elastic decoherence rates.
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- In this study, we apply the monitoring master equation describing decoherence of internal states to an optically active molecule prepared in a coherent superposition of...
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