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Open Quantum Systems Decoherence Quantum Chemistry

Enhancing the intense field control of molecular fragmentation

arXiv
Authors: Fatima Anis, B. D. Esry

Year

2011

Paper ID

29439

Status

Preprint

Abstract Read

~2 min

Abstract Words

59

Citations

N/A

Abstract

We describe a pump-probe scheme with which the spatial asymmetry of dissociating molecular fragments --- as controlled by the carrier-envelope phase of an intense few-cycle laser pulse --- can be enhanced by an order of magnitude or more. We illustrate the scheme using extensive, full-dimensional calculations for dissociation of H2^+ and include the averaging necessary for comparison with experiment.

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  • We describe a pump-probe scheme with which the spatial asymmetry of dissociating molecular fragments --- as controlled by the carrier-envelope phase of an intense few-cycle...

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