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Nuclear classical dynamics of H2 in intense laser field

arXiv
Authors: Firoozeh Sami, Mohsen Vafaee, Babak Shokri

Year

2010

Paper ID

28918

Status

Preprint

Abstract Read

~2 min

Abstract Words

217

Citations

N/A

Abstract

In the first part of this paper, the different distinguishable pathways and regions of the single and sequential double ionization are determined and discussed. It is shown that there are two distinguishable pathways for the single ionization and four distinct pathways for the sequential double ionization. It is also shown that there are two and three different regions of space which are related to the single and double ionization respectively. In the second part of the paper, the time dependent Schrödinger and Newton equations are solved simultaneously for the electrons and the nuclei of H2 respectively. The electrons and nuclei dynamics are separated on the base of the adiabatic approximation. The soft-core potential is used to model the electrostatic interaction between the electrons and the nuclei. A variety of wavelengths (390 nm, 532 nm and 780 nm) and intensities $5times1014$ $Wcm-2 $ and $ 5times1015$ $Wcm-2$ of the ultrashort intense laser pulses with a sinus second order envelope function are used. The behaviour of the time dependent classical nuclear dynamics in the absence and present of the laser field are investigated and compared. In the absence of the laser field, there are three distinct sections for the nuclear dynamics on the electronic ground state energy curve. The bond hardening phenomenon does not appear in this classical nuclear dynamics simulation.

Why This Paper Matters

  • This paper contributes to the Quantum Simulation research area in the Quantum Articles archive.
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  • In the first part of this paper, the different distinguishable pathways and regions of the single and sequential double ionization are determined and discussed.

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