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Quantum Chemistry

Ultralong-Range Rb-KRb Rydberg Molecules: Selected Aspects of Electronic Structure, Orientation and Alignment

arXiv
Authors: Javier Aguilera-Fernández, H. R. Sadeghpour, Peter Schmelcher, Rosario González-Férez

Year

2015

Paper ID

27881

Status

Preprint

Abstract Read

~2 min

Abstract Words

110

Citations

N/A

Abstract

We investigate the structure and features of an ultralong-range triatomic Rydberg molecule formed by a Rb Rydberg atom and a KRb diatomic molecule. In our numerical description, we perform a realistic treatment of the internal rotational motion of the diatomic molecule, and take into account the Rb$n, lge 3$ Rydberg degenerate manifold and the energetically closest neighboring levels with principal quantum numbers n'>n and orbital quantum number lle2. We focus here on the adiabatic electronic potentials evolving from the Rb$n, lge 3$ and Rb$n=26, l=2$ manifolds. The directional properties of the KRb diatomic molecule within the Rb-KRb triatomic Rydberg molecule are also analyzed in detail.

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  • We investigate the structure and features of an ultralong-range triatomic Rydberg molecule formed by a Rb Rydberg atom and a KRb diatomic molecule.

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References & Citation Signals

[1] DOI https://doi.org/arXiv:1507.07972 [2] arXiv https://arxiv.org/abs/1507.07972 [3] Publisher https://arxiv.org/abs/1507.07972

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